The 1870 census for Andover, NH, has the 15-year-old Frank working as a farm hand in the household of Oscar and Lucy Eastman.
Frank Sylvester Bartlett married Carrie Minerva Emerson on July 4, 1875 in Andover NH. Eastman: History of Andover NH (online at openlibrary.org). Apparently no children were born to Frank and Carrie (census 1900 & 1910, family records).
Frank can be found in the US Censuses until 1930. One the picture scans of an August, 1938 Bartlett reunion has Frank in it.
"New Hampshire Birth Records, Early to 1900," database with images, FamilySearch (https://familysearch.org/ark:/61903/1:1:FL2F-DPG : 8 April 2020), Frank S Bartlett, 09 Feb 1854; citing East Kingston, Rockingham, New Hampshire, United States, Bureau of Vital Records and Health Statistics, Concord; FHL microfilm 1,000,371.
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It may be possible to confirm family relationships with Frank by comparing test results with other carriers of his ancestors' Y-chromosome or mitochondrial DNA.
However, there are no known yDNA or mtDNA test-takers in his direct paternal or maternal line.
It is likely that these autosomal DNA test-takers will share some percentage of DNA with Frank: