Appears to have passed away prior to 1891 census; appears on 1861, 1871, and 1881 censuses, but wife Elizabeth is listed as a widow on the 1891 census.
Sources
p.540 of 'Rawdon and Douglas: Two Loyalist townships in Nova Scotia' by John V Duncanson
https://central.bac-lac.gc.ca/.item/?app=Census1861&op=img&id=4108904_00572 - 4 males, 6 females in house (all single except noted below): 1 female <1 year old; 2 females over 5 years and under 10 years old; 1 male and 1 female over 10 years and under 15 years old; 1 female over 15 years and under 20 years old; 2 males over 20 years and under 30 years old; 1 male and 1 female (both married) over 40 years and under 50 years old. 2 females over 5 years and under 15 years old who cannot read; 2 females over 5 years and under 15 years old who cannot write (presumably the same two).
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DNA Connections
It may be possible to confirm family relationships with Samuel by comparing test results with other carriers of his Y-chromosome or his mother's mitochondrial DNA.
However, there are no known yDNA or mtDNA test-takers in his direct paternal or maternal line.
It is likely that these autosomal DNA test-takers will share some percentage of DNA with Samuel:
Singer-1639 and Singer-583 appear to represent the same person because: Daniel Singer is from Lattiesbrook. His marriage in NS BMD shows his father to be Samuel. DNA shows a connection to Singers from Singer 538. This is the only Samuel Singer I can find about the correct age.